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Abstract. Most global aerosol models approximate dust as sphericalparticles, whereas most remote sensing retrieval algorithms approximate dust as spheroidal particles with a shape distribution that conflicts withmeasurements. These inconsistent and inaccurate shape assumptions generatebiases in dust single-scattering properties. Here, we obtain dustsingle-scattering properties by approximating dust as triaxial ellipsoidalparticles with observationally constrained shape distributions. We findthat, relative to the ellipsoidal dust optics obtained here, the sphericaldust optics used in most aerosol models underestimate dust single-scattering albedo, mass extinction efficiency, and asymmetry parameter for almost all dust sizes in both the shortwave and longwave spectra. We further find that the ellipsoidal dust optics are in substantially better agreement with observations of the scattering matrix and linear depolarization ratio than the spheroidal dust optics used in most retrieval algorithms. However, relative to observations, the ellipsoidal dust optics overestimate the lidar ratio by underestimating the backscattering intensity by a factor of ∼2. This occurs largely because the computational method used to simulate ellipsoidal dust optics (i.e., the improved geometric optics method) underestimates the backscattering intensity by a factor of ∼2 relative to other computational methods (e.g., the physical geometric optics method). We conclude that the ellipsoidal dust optics with observationally constrained shape distributions can help improve global aerosol models and possibly remote sensing retrieval algorithms that do not use the backscattering signal. 

ABSTRACT The size of dust grains, a, is key to the physical and chemical processes in circumstellar discs, but observational constraints of grain size remain challenging. (Sub)millimetre continuum observations often show a per cent-level polarization parallel to the disc minor axis, which is generally attributed to scattering by $${\sim}100\, \mu{\rm m}$$-sized spherical grains (with a size parameter x ≡ 2$$\pi$$a/λ < 1, where λ is the wavelength). Larger spherical grains (with x greater than unity) would produce opposite polarization direction. However, the inferred size is in tension with the opacity index β that points to larger mm/cm-sized grains. We investigate the scattering-produced polarization by large irregular grains with a range of x greater than unity with optical properties obtained from laboratory experiments. Using the radiation transfer code, RADMC-3D, we find that large irregular grains still produce polarization parallel to the disc minor axis. If the original forsterite refractive index in the optical is adopted, then all samples can produce the typically observed level of polarization. Accounting for the more commonly adopted refractive index using the DSHARP dust model, only grains with x of several (corresponding to ∼mm-sized grains) can reach the same polarization level. Our results suggest that grains in discs can have sizes in the millimetre regime, which may alleviate the tension between the grain sizes inferred from scattering and other means. Additionally, if large irregular grains are not settled to the mid-plane, their strong forward scattering can produce asymmetries between the near and far side of an inclined disc, which can be used to infer their presence.